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Abstract. Scattering codes are used to study the optical properties of polar stratospheric clouds (PSCs). Particle backscattering and depolarization coefficients can be computed with available scattering codes once the particle size distribution (PSD) is known and a suitable refractive index is assumed. However, PSCs often appear as external mixtures of supercooled ternary solution (STS) droplets, solid nitric acid trihydrate (NAT) and possibly ice particles, making the assumption of a single refractive index and a single morphology to model the scatterers questionable.Here we consider a set of 15 coincident measurements of PSCs above McMurdo Station, Antarctica, using ground-based lidar, a balloon-borne optical particle counter (OPC) and in situ observations taken by a laser backscattersonde and OPC during four balloon stratospheric flights from Kiruna, Sweden. This unique dataset of microphysical and optical observations allows us to test the performances of optical scattering models when both spherical and aspherical scatterers of different composition and, possibly, shapes are present. We consider particles as STS if their radius is below a certain threshold value Rth and NAT or possibly ice if it is above it. The refractive indices are assumed known from the literature. Mie scattering is used for the STS, assumed spherical. Scattering from NAT particles, considered spheroids of different aspect ratio (AR), is treated with T-matrix results where applicable. The geometric-optics–integral-equation approach is used whenever the particle size parameter is too large to allow for a convergence of the T-matrix method.The parameters Rth and AR of our model have been varied between 0.1 and 2 µm and between 0.3 and 3, respectively, and the calculated backscattering coefficient and depolarization were compared with the observed ones. The best agreement was found for Rth between 0.5 and 0.8 µm and for AR less than 0.55 and greater than 1.5.To further constrain the variability of AR within the identified intervals, we have sought an agreement with the experimental data by varying AR on a case-by-case basis and further optimizing the agreement by a proper choice of AR smaller than 0.55 and greater than 1.5 and Rth within the interval 0.5 and 0.8 µm. The ARs identified in this way cluster around the values 0.5 and 2.5.The comparison of the calculations with the measurements is presented and discussed. The results of this work help to set limits to the variability of the dimensions and asphericity of PSC solid particles, within the limits of applicability of our model based on the T-matrix theory of scattering and on assumptions on a common particle shape in a PSD and a common threshold radius for all the PSDs. 

Abstract. A novel fiber-optic distributed temperature sensing instrument, the Fiber-optic Laser Operated Atmospheric Temperature Sensor (FLOATS), was developed for continuous in situ profiling of the atmosphere up to 2 km below constant-altitude scientific balloons. The temperature-sensingsystem uses a suspended fiber-optic cable and temperature-dependent scattering of pulsed laser light in the Raman regime to retrieve continuous3 m vertical-resolution profiles at a minimum sampling period of 20 s.FLOATS was designed for operation aboard drifting super-pressure balloons inthe tropical tropopause layer at altitudes around 18 km as part of theStratéole 2 campaign. A short test flight of the system was conductedfrom Laramie, Wyoming, in January 2021 to check the optical, electrical, andmechanical systems at altitude and to validate a four-reference temperaturecalibration procedure with a fiber-optic deployment length of 1170 m. During the 4 h flight aboard a vented balloon, FLOATS retrieved temperatureprofiles during ascent and while at a float altitude of about 19 km. TheFLOATS retrievals provided differences of less than 1.0 ∘Ccompared to a commercial radiosonde aboard the flight payload during ascent.At float altitude, a comparison of optical length and GPS position at thebottom of the fiber-optic revealed little to no curvature in the fiber-opticcable, suggesting that the position of any distributed temperaturemeasurement can be effectively modeled. Comparisons of the distributed temperature retrievals to the reference temperature sensors show strongagreement with root-mean-square-error values less than 0.4 ∘C. Theinstrument also demonstrated good agreement with nearby meteorologicalobservations and COSMIC-2 satellite profiles. Observations of temperatureand wind perturbations compared to the nearby radiosounding profiles provide evidence of inertial gravity wave activity during the test flight. Spectral analysis of the observed temperature perturbations shows that FLOATS is an effective and pioneering tool for the investigation of small-scale gravity waves in the upper troposphere and lower stratosphere. 

Profiles of stratospheric aerosol size distributions have been measured using balloon‐bornein situoptical particle counters, from Laramie, Wyoming (41°N) since 1971. In 2019, this measurement record transitioned to the Laboratory for Atmospheric and Space Physics (LASP) in Boulder, Colorado (40°N). The new LASP Optical Particle Counter (LOPC), the fourth generation of instruments used for this record, is smaller and lighter (2 kg) than prior instruments, measures aerosols with diameters ≥0.3–30 μm in up to 450 size bins, with a flow rate of 20 L min⁻¹. The improved size resolution enables the complete measurement of size distributions, and calculation of aerosol extinction without fittinga prioridistribution shapes. The higher flow provides the sensitivity required to measure super‐micron particles in the stratosphere. The LOPC has been validated against prior Wyoming OPCs, through joint flights, laboratory comparisons, and statistical comparisons with the Wyoming record. The agreement between instruments is generally within the measurement uncertainty of ±10%–20% in sizing and ±10% in concentration, and within ±40% for calculated aerosol moments. The record is being continued with balloon soundings every 2 months from Colorado, coordinated with measurements of aerosol extinction from the SAGE III instrument on the International Space Station. Comparisons of aerosol extinction from the remote andin situplatforms have shown good agreement in the stratosphere, particularly for wavelengths <755 nm and altitudes <25 km. For extinction wavelengths ≥1,021 nm and altitudes above 25 km SAGE III/International Space Station extinction has a low bias relative to thein situmeasurements, yet still within the ±40% uncertainty.

 

Abstract. The tropical tropopause layer (TTL; 14–18.5 km) is the gateway formost air entering the stratosphere, and therefore processes within thislayer have an outsized influence in determining global stratospheric ozoneand water vapor concentrations. Despite the importance of this layer thereare few in situ measurements with the necessary detail to resolve the fine-scale processes within this region. Here, we introduce a novel platform forhigh-resolution in situ profiling that lowers and retracts a suspendedinstrument package beneath drifting long-duration balloons in the tropics.During a 100 d circumtropical flight, the instrument collected over a hundred 2 km profiles of temperature, water vapor, and aerosol at 1 m resolution, yielding unprecedented geographic sampling and verticalresolution. The instrument system integrates proven sensors for water vapor,temperature, pressure, and cloud and aerosol particles with an innovativemechanical reeling and control system. A technical evaluation of the systemperformance demonstrated the feasibility of this new measurement platformfor future missions with minor modifications. Six instruments planned fortwo upcoming field campaigns are expected to provide over 4000 profilesthrough the TTL, quadrupling the number of high-resolution aircraft andballoon profiles collected to date. These and future measurements willprovide the necessary resolution to diagnose the importance of competingmechanisms for the transport of water vapor across the TTL. 

Abstract. A comparison of polar stratospheric cloud (PSC) occurrence from 2006 to2010 is presented, as observed from the ground-based lidar station at McMurdo(Antarctica) and by the satellite-borne CALIOP lidar (Cloud-Aerosol Lidarwith Orthogonal Polarization) measuring over McMurdo. McMurdo (Antarctica) isone of the primary lidar stations for aerosol measurements of the NDACC (Network forDetection of Atmospheric Climate Change). The ground-based observations havebeen classified with an algorithm derived from the recent v2 detection andclassification scheme, used to classify PSCs observed by CALIOP.

A statistical approach has been used to compare ground-based and satellite-based observations, since point-to-point comparison is often troublesome dueto the intrinsic differences in the observation geometries and the imperfectoverlap of the observed areas.

A comparison of space-borne lidar observations and a selection of simulationsobtained from chemistry–climate models (CCMs) has been made by using a series ofquantitative diagnostics based on the statistical occurrence of different PSCtypes. The distribution of PSCs over Antarctica, calculated by severalCCMVal-2 and CCMI chemistry–climate models has been compared with the PSCcoverage observed by the satellite-borne CALIOP lidar. The use of severaldiagnostic tools, including the temperature dependence of the PSCoccurrences, evidences the merits and flaws of the different models. Thediagnostic methods have been defined to overcome (at least partially) thepossible differences due to the resolution of the models and to identifydifferences due to microphysics (e.g., the dependence of PSC occurrence onT−T_NAT).

A significant temperature bias of most models has been observed, as well as alimited ability to reproduce the longitudinal variations in PSC occurrencesobserved by CALIOP. In particular, a strong temperature bias has been observedin CCMVal-2 models with a strong impact on PSC formation. The WACCM-CCMI(Whole Atmosphere Community Climate Model – Chemistry-Climate ModelInitiative) model compares rather well with the CALIOP observations, althougha temperature bias is still present.

 

Atmospheric waves in the tropical tropopause layer are recognized as a significant influence on processes that impact global climate. For example, waves drive the quasi‐biennial oscillation (QBO) in equatorial stratospheric winds and modulate occurrences of cirrus clouds. However, the QBO in the lower stratosphere and thin cirrus have continued to elude accurate simulation in state‐of‐the‐art climate models and seasonal forecast systems. We use first‐of‐their‐kind profile measurements deployed beneath a long‐duration balloon to provide new insights into impacts of fine‐scale waves on equatorial cirrus clouds and the QBO just above the tropopause. Analysis of these balloon‐borne measurements reveals previously uncharacterized fine‐vertical‐scale waves (<1 km) with large horizontal extent (>1000 km) and multiday periods. These waves affect cirrus clouds and QBO winds in ways that could explain current climate model shortcomings in representing these stratospheric influences on climate. Accurately simulating these fine‐vertical‐scale processes thus has the potential to improve sub‐seasonal to near‐term climate prediction.

 

In the Stratéole 2 program, set to launch in November 2018, instruments will ride balloons into the stratosphere and circle the world, observing properties of the air and winds in fine detail. 

Macroscopic stratospheric aerosol properties such as surface area density (SAD) and volume density (VD) are required by modern chemistry climate models. These quantities are in continuous need of validation by observations. Direct observation of these parameters is not possible, but they can be derived from optical particle counters (OPCs) which provide concentration (number density) and size distributions of aerosol particles, and possibly from ground‐based and satellite‐borne lidar observations of particle backscatter coefficients and aerosol type. When such measurements are obtained simultaneously by OPCs and lidars, they can be used to calculate backscatter and extinction coefficients, as well as SAD and VD. Empirical relations can thus be derived between particle backscatter coefficient, extinction coefficient, and SAD and VD for a variety of aerosols (desert dust, maritime aerosols, stratospheric aerosols) and be used to approximate SAD and VD from lidar measurements. Here we apply this scheme to coincident measurements of polar stratospheric clouds above McMurdo Station, Antarctica, by ground‐based lidar and balloon‐borne OPCs. The relationships derived from these measurements will provide a means to obtain values of SAD and VD for supercooled ternary solutions (STS) and nitric acid trihydrate (NAT) PSCs from the backscatter coefficients measured by lidar. Coincident lidar and OPC measurements provided 15 profile comparisons. Empirical expressions of SAD and VD as a function of particle backscatter coefficient,β, were calculated from fits of the form log(SAD/VD) = A + Blog(β) usingβfrom the lidar and SAD/VD from the OPC. The PSCs were classified as STS and NAT mixtures, ice being absent.

 

The method to derive aerosol size distributions from in situ stratospheric measurements from the University of Wyoming is modified to include an explicit counting efficiency function (CEF) to describe the channel‐dependent instrument counting efficiency. This is motivated by Kovilakam and Deshler's (2015,https://doi.org/10.1002/2015JD023303) discovery of an error in the calibration method applied to the optical particle counter (OPC40) developed in the late 1980s and used from 1991 to 2012. The method can be applied to other optical aerosol instruments for which counting efficiencies have been measured. The CEF employed is the integral of the Gaussian distribution representing the instrument response at any one aerosol channel, the aerosol counting efficiency. Results using the CEF are compared to previous derivations of aerosol size distributions (Deshler et al., 2003,https://doi.org/10.1029/2002JD002514) applied to the measurements before and after Kovilakam and Deshler's correction of number concentration for the OPC40 calibration error. The CEF method is found, without any tuning parameter, to reproduce or improve upon the Kovilakam and Deshler's results, thus accounting for the calibration error without any external comparisons other than the laboratory determined counting efficiency at each aerosol channel. Moments of the new aerosol size distributions compare well with aerosol extinctions measured by Stratospheric Aerosol and Gas Experiment II and Halogen Occultation Experiment in the volcanic period 1991–1996, generally within ±40%, the precision of OPC40 moments, and in the nonvolcanic period after 1996, generally within ±20%. Stratospheric Aerosol and Gas Experiment II and Halogen Occultation Experiment estimates of aerosol surface area are generally in agreement with those derived using the new CEF method.